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Symmetry Breaking, Order-by-Disorder, Fragmentation, and Spin-Liquids in the Magnetic Pyrochlore Lattice with Anisotropic Interactions

dc.contributor.authorLozano Gomez, Daniel
dc.date.accessioned2023-01-26T21:19:33Z
dc.date.issued2023-01-26
dc.date.submitted2023-01-26
dc.description.abstractWithin the study of frustrated magnetism, the pyrochlore lattice is deemed a fruitful ground where phenomena such as quantum and thermal order-by-disorder, moment fragmentation, and spin-liquids, both quantum and classical, might be realized. In this thesis, we study a Heisenberg and Dzyaloshisnkii-Moriya nearest-neighbor Hamiltonian in this lattice which presents all the above phenomena, providing a quantitative description through the application of both analytical and numerical approaches. First, we obtain a phase diagram where three long-range ordered phases (two antiferromagnetic and one ferromagnetic), and two spin-liquid points, the well-known classical Coulomb phase and a new spin-liquid, that we dub “order-by-disorder selected spin liquid”, are identified. We then proceed to study the order-by-disorder selection in two of the long-range ordered phases (an antiferromagnetic and a ferromagnetic phase) and show that the quantum order-by-disorder selection mechanism in one of these phases is only produced at non-zero temperature, i.e. without zero-temperature quantum order-by-disorder. Then, we study the newly identified spin-liquid and the evolution of its correlation function as a function of temperature. The correlation function of this spin-liquid presents pinch-lines, twofold and fourfold pinch-points at high temperature, whereas at low temperature, these features are replaced by a spin-ice pattern. This effect is a consequence of the order-by-disorder selection of an extensive subset of ground-states (the spin-ice states) within the manifold. Finally, we study the phenomenon of fragmentation, commonly referred to as the observation of both sharp pinch-points and Bragg peaks in the correlation functions of an ordered phase. Specifically, we demonstrate how this effect is a consequence of a Helmholtz-Hodge decomposition of the spin mode excitations in an ordered phase, and is therefore expected to be observed especially for Hamiltonians whose interaction parameters are proximate to a spin-liquid point.en
dc.identifier.urihttp://hdl.handle.net/10012/19133
dc.language.isoenen
dc.pendingfalse
dc.publisherUniversity of Waterlooen
dc.relation.urihttps://github.com/daniel-lozano/Thesis_animationsen
dc.subjectfrustrated magnetismen
dc.subjectorder by disorderen
dc.subjectspin liquiden
dc.subjectpyrochlore latticeen
dc.titleSymmetry Breaking, Order-by-Disorder, Fragmentation, and Spin-Liquids in the Magnetic Pyrochlore Lattice with Anisotropic Interactionsen
dc.typeDoctoral Thesisen
uws-etd.degreeDoctor of Philosophyen
uws-etd.degree.departmentPhysics and Astronomyen
uws-etd.degree.disciplinePhysicsen
uws-etd.degree.grantorUniversity of Waterlooen
uws-etd.embargo2025-01-25T21:19:33Z
uws-etd.embargo.terms2 yearsen
uws.contributor.advisorGingras, Michel
uws.contributor.affiliation1Faculty of Scienceen
uws.peerReviewStatusUnrevieweden
uws.published.cityWaterlooen
uws.published.countryCanadaen
uws.published.provinceOntarioen
uws.scholarLevelGraduateen
uws.typeOfResourceTexten

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